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Reasons from decay-corrected activity ledgers, decay modes and cross sections, and ALARA dose control through Bateman/ORIGEN modeling, extraction-chromatography separations (TRU/Sr/TEVA resins), and HPGe/alpha/LSC spectroscopy while treating daughter ingrowth, generator breakthrough, spectral pile-up and sum peaks, and swipe-test cross-contamination as first-class failure modes.